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Perhaps not too much of a doozy, but you'll want to be careful.
By virtue of leasing a car to the business, she becomes a de facto sole proprietorship (business) herself.
That means depreciating the car, accounting for maintenance, oil, registration, taxes, interest, etc. and reporting it on Schedule C. She cannot deduct car payments. She can only deduct the interest portion of those car payments.
She will need to apportion the costs based on the time she drives it and the LLC uses it. She can use mileage for the apportionment factor. She might be able to just use the standard mileage rate (currently $0.50/mile, I think) for any miles used by the LLC in lieu of accounting and keeping track of all the other costs.
You will need to have a very clear contract between her and the LLC for the lease.